标题:Effect of pH on the adsorption and photocatalytic degradation of sulfadimidine in Vis/g-C3N4 progress作者:Yang, B (Yang, Bin); Mao, XH (Mao, Xuhui); Pi, L (Pi, Liu); Wu, YX (Wu, Yixiao); Ding, HJ (Ding, Huijun); Zhang, WH (Zhang, Weihao)
来源出版物:ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH卷:24期:9 页码:8658-8670 DOI:10.1007/s11356-017-8448-0 出版年:MAR 2017
摘要: In this study, g-C3N4 was synthesized by thermal polycondensation of melamine and was characterized by X-ray powder diffraction, X-ray photoelectron spectroscopy, UV-visible diffuse reflection spectroscopy, and scanning electron microscopy. Results showed that g-C3N4 degraded sulfadimidine (SMD) under visible light, in which the adsorption and photocatalytic degradation was influenced by pH. The maximum adsorption capacity was achieved at approximately pH 5. The highest degradation rate constant was obtained at strong acid and alkali. In addition, the degradation mechanism of g-C3N4 was evaluated with the help of quencher agents. The intermediates, degradation pathways, and mineralization of SMD were also determined to evaluate the degradation and oxidation ability of g-C3N4.
入藏号:WOS:000399162900073
文献类型:Article
语种:English
作者关键词: Antibiotics; g-C3N4; Degradation pathways; Photodegradation
扩展关键词: CARBON NANOTUBES; HETEROCYCLIC GROUPS; ACTIVATED CARBON; NATURAL-WATERS; SULFA DRUGS; G-C3N4; PHOTODEGRADATION; ANTIBIOTICS; PHOTOLYSIS; OXIDATION
通讯作者地址:Zhang, WH (reprint author), Wuhan Univ, Coll Resource & Environm Sci, Wuhan 430072, Peoples R China.
Zhang, WH (reprint author), Wuhan Univ, Hubei Prov Collaborat Innovat Ctr Water Resources, Wuhan 430072, Peoples R China.
电子邮件地址: zhangwh@whu.edu.cn
地址:
[Yang, Bin; Mao, Xuhui; Pi, Liu; Wu, Yixiao; Ding, Huijun; Zhang, Weihao] Wuhan Univ, Coll Resource & Environm Sci, Wuhan 430072, Peoples R China.
[Zhang, Weihao] Wuhan Univ, Hubei Prov Collaborat Innovat Ctr Water Resources, Wuhan 430072, Peoples R China.
研究方向:Environmental Sciences & Ecology
ISSN: 0944-1344
eISSN:1614-7499
影响因子:2.76
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