标题:Fine particles (PM2.5) at a CAWNET background site in Central China: Chemical compositions, seasonal variations and regional pollution events作者:Zhang, Fan; Cheng, Hai-rong; Wang, Zu-wu; Lv, Xiao-pu; Zhu, Zhong-min;Zhang, Gan; Wang, Xin-ming
来源出版物:ATMOSPHERIC ENVIRONMENT 卷:86 页:193-202 DOI:10.1016/j.atmosenv.2013.12.008 出版年:APR 2014
摘要:Fine particle (PM2.5) samples were collected at Jinsha (JSH), a regional background China Atmosphere Watch Network (CAWNET) site in Central China from March 2012 to March 2013. The mass concentrations of water-soluble inorganic ions (WSIIs), organic carbon (OC) and elemental carbon (EC) in PM2.5 were measured. The average PM2.5 mass concentration was 48.7 +/- 26.9 mu g m(-3), exceeding the Chinese National Ambient Air Quality Standards (NAAQS) (35 mu g m(-3)), implying that PM2.5 is a pollutant of regional concern in Central China. The average concentrations of total WSIls, OC and EC were 26.1 +/- 18.8, 7.5 +/- 3.5 and 0.7 +/- 0.5 mu g m(-3), accounting for 53.5%, 15.1% and 1.5% of the PM2.5 concentrations at JSH, respectively. Clear seasonal variations in PM2.5 and the levels of its main chemical species were observed in the following order: winter > autumn > spring > summer. Backward air trajectory analysis and potential source contribution function (PSCF) analysis implied that the areas north and northeast of JSH contributed significantly to the levels of SO42-, NO3-, NH4+ and OC, while sandstorms originating from Mongolia and traveling across Northwest China may have contributed significantly to the levels of Na+, Ca2+, and Mg2+ in PM2.5 at JSH. Two pollution events, related to regional biomass burning and haze, respectively, were recorded at JSH during the sampling campaign.
入藏号:WOS:000332143100022
文献类型:Article
语种:English
作者关键词:PM2.5, Background, Long-range atmospheric transport, Back trajectory, Potential source contribution function (PSCF), Pollution events
扩展关键词:LONG-RANGE TRANSPORT; CARBONACEOUS AEROSOLS; ORGANOCHLORINE PESTICIDES; SOUTHERN CALIFORNIA; NORTHWESTERN CHINA; PARTICULATE MATTER; ORGANIC-COMPOUNDS; WESTERN CHINA; GAW STATION; AMBIENT AIR
通讯作者地址:Cheng, Hai-rong; Wuhan Univ, Sch Resource & Environm Sci, Dept Environm Engn, Wuhan 430069, Peoples R China.
电子邮件地址:chenghr@whu.edu.cn
地址:
[Zhang, Fan; Cheng, Hai-rong; Wang, Zu-wu; Lv, Xiao-pu]Wuhan Univ, Sch Resource & Environm Sci, Dept Environm Engn, Wuhan 430069, Peoples R China.
[Zhang, Gan; Wang, Xin-ming] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China.
[Zhu, Zhong-min] Huazhong Univ Sci & Technol, Wuchang Branch, Wuhan 430064, Peoples R China.
研究方向:Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences
ISSN:1352-2310
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