1.标题:Removal of sulfamethoxazole from aqueous solution by sono-ozonation in the presence of a magnetic catalyst作者:Hou, Liwei; Zhang, Hui; Wang, Liguo; Chen, Lu; Xiong, Yidong; Xue,Xiaofei
来源出版物:SEPARATION AND PURIFICATION TECHNOLOGY 卷:117 特刊:SI 页:46-52 DOI:10.1016/j.seppur.2013.05.014 出版年:SEP 30 2013
摘要:The degradation of sulfamethoxazole (SMX) was investigated under the sono-catalytic ozonation process over magnetic suspension. The effects of various operating conditions were investigated, including initial pH value, catalyst dosage, and power density. The results indicated that the degradation of SMX followed a pseudo-first-order kinetic model under different operating conditions. The removal rate increased with the increase of pH, but it decreased when the catalyst dosage or power density exceeded a certain value. The removal rate was inhibited in the presence of tert-butyl alcohol, isopropanol or NaF. After 20 min treatment, the COD removal reached 57.5%, the acute toxicity to Daphnia magna largely decreased, and the biodegradability (BOD5/COD ratio) increased from 0.02 to 0.41. COD was almost completely removed when the reaction time was extended to 120 min.
入藏号:WOS:000324604000009
文献类型:Article
语种:English
作者关键词:Sulfamethoxazole, Sono-catalytic ozonation, Magnetic, Acute toxicity, Biodegradability
扩展关键词:RECTANGULAR AIRLIFT REACTOR; DYE ORANGE-II; ULTRASONIC IRRADIATION; FENTON PROCESS; WASTE-WATER; DEGRADATION; OZONE; ACID; DECOMPOSITION; KINETICS
通讯作者地址:Zhang, Hui; Wuhan Univ, Hubei Biomass Resource Chem & Environm Biotechnol, Dept Environm Engn, Wuhan 430079, Peoples R China.
电子邮件地址:eeng@whu.edu.cn
地址:
[Hou, Liwei; Zhang, Hui; Wang, Liguo; Chen, Lu; Xue, Xiaofei] Wuhan Univ, Hubei Biomass Resource Chem & Environm Biotechnol, Dept Environm Engn, Wuhan 430079, Peoples R China.
[Xiong, Yidong] Wuhan Univ, Sch Phys & Technol, Wuhan 430072, Peoples R China.
研究方向:Engineering
ISSN:1383-5866
2.标题:Degradation of bisphenol A in aqueous solution by a novel electro/Fe3+/peroxydisulfate process作者:Lin, Heng; Wu, Jie; Zhang, Hui
来源出版物:SEPARATION AND PURIFICATION TECHNOLOGY 卷:117特刊:SI页:18-23 DOI:10.1016/j.seppur.2013.04.026出版年:SEP 30 2013
摘要: The removal of bisphenol A (BPA) by a novel "electro/Fe3+/peroxydisulfate" process is reported in this study. The effects of initial pH, electrolyte concentration, Fe3+ concentration, peroxydisulfate (PDS) concentration and current density were investigated. The results indicated that the removal efficiency of BPA declined with the increase of initial pH and electrolyte concentration, but increased with an increase of Fe3+ concentration and current density. The BPA degradation efficiency was improved significantly when the PDS concentration was increased from 1 to 10 mM, but further PDS increase had little effect. BPA was almost completely removed after 60 min reaction and a TOC removal efficiency of 94.3% was achieved when the reaction time was extended to 120 min.
入藏号:WOS:000324604000004
文献类型:Article
语种:English
作者关键词:Bisphenol A, Electrochemical oxidation, Ferric iron, Peroxydisulfate, Sulfate radicals
扩展关键词:ACID ORANGE 7; ACTIVATED PERSULFATE OXIDATION; GENERATED FENTONS REAGENT; BORON-DOPED DIAMOND; 2,4,5-TRICHLOROPHENOXYACETIC ACID; PERFLUOROCARBOXYLIC ACIDS; EFFICIENT DECOMPOSITION; WATER DECONTAMINATION; HYDROGEN-PEROXIDE; ANODIC-OXIDATION
通讯作者地址:Zhang, Hui; Wuhan Univ, Hubei Biomass Resource Chem & Environm Biotechnol, Dept Environm Engn, Wuhan 430079, Peoples R China.
电子邮件地址:eeng@whu.edu.cn
地址:
[Lin, Heng; Wu, Jie; Zhang, Hui] Wuhan Univ, Hubei Biomass Resource Chem & Environm Biotechnol, Dept Environm Engn, Wuhan 430079, Peoples R China.
研究方向:Engineering
ISSN:1383-5866
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